Synthesis of water-stable and highly luminescent graphite quantum dots

Slavia Deeksha Dsouza, Marius Buerkle, Bruno Alessi, Paul Brunet, Alessio Morelli, Amir Farokh Payam, Paul Maguire, Davide Mariotti, Vladimir Svrcek

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Highly stable and environmentally friendly nitrogen-doped graphite quantum dots consisting of ~12 layers of graphene, average diameter of ~7.3 nm, prepared by atmospheric pressure microplasma are reported to have blue emission due to surface states created by nitrogen doping (9 atomic%) and reaction with oxygen. The low-temperature synthesis method requires simple precursors in water, with no annealing or filtration, producing crystalline disc-shaped quantum dots with ~68 % photoluminescence emission quantum yield at 420 nm excitation and that have shown stability for more than one month after the synthesis. The nitrogen doping in the quantum dots mainly occurs in graphitic core as substituted type of doping (63-67 atomic%) and the amount of doping is sufficient to create emissive states without impacting the core structure. The optical and chemical properties do not undergo serious retardation even with re-dispersion suggesting easy applicability for cellular imaging or optoelectronics. [Abstract copyright: Creative Commons Attribution license.]
Original languageEnglish
Issue number50
Early online date8 Sept 2023
Publication statusPublished online - 8 Sept 2023

Bibliographical note

Publisher Copyright:
Creative Commons Attribution license.


  • doping
  • electro-optical materials
  • colloids
  • blue luminescence
  • atmospheric pressure microplasma


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